I'd stay as dry as possible. Drysuit, dry gloves, FFM for at least parts of the dive. I would also do a mix of swimming and sitting. You'll want at least two big slates, one for you to use and the other to be cleaned off for you to use later. If you get an FFM (which you should) then I recommend splurging for the comms unit as well. You'll want a heating vest with IO connector for recharging mid-dive. You'll want a few good lights, even if they're on the boat pointing down.
I would recommend doing it somewhere near a recompression chamber, I recommend informing them of your stunt beforehand, and I recommend you calling DAN a good, long while before hand. I think DAN might have some good insights. Also, purchase DAN insurance. The nicest one there is. Heck, buy two if they'll let you
. Also, doing a combination of nitrox and air isn't a bad idea. Switching between higher O2 percentages for reduced nitrogen ongassing, and then as low of O2 as you can go (maybe He?) just to reduce O2 accumulation.
For entertainment, there are underwater iPhone cases that can be used for movies. Also, iPod shuffles can be had for cheap that have been waterproofed to a good depth and designed for this kinda thing (sort of).
I might recommend setting up some "challenges"....like swimming through loops. Playing chess/checkers with someone. Maybe a speargun and some targets for target practice. You're going to be CRAZY bored for 72 hours.
Logistics: I did some rough calculations, and you're going to need somewhere near 7000 ft3 of gas for those 72 hours. I mean, that's 110 AL80's breathed from 3000psi to 500psi. I recommend sidemount for those logistics, and having your support crew clipping and unclipping the tanks. That or doubles, and just switching between bcd's.....which I feel like would be taxing. Have you run the calculations as far as deco requirements and CNS stuff goes? EAN32 gives you deco of like 9 hours according to DecoPlanner. EAN36 gives you no deco, but means your CNS% will be pushing 1000%. What are your feelings on this kind of logistics?
Most importantly: If you do this, PM me about diving support for you. I would be proud to volunteer time and gear for prep and/or the real dive.